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Journal Articles

Study on chemical form of tritium in coolant helium of high temperature gas-cooled reactor with tritium production device

Hamamoto, Shimpei; Ishitsuka, Etsuo; Nakagawa, Shigeaki; Goto, Minoru; Matsuura, Hideaki*; Katayama, Kazunari*; Otsuka, Teppei*; Tobita, Kenji*

Proceedings of 2021 International Congress on Advances in Nuclear Power Plants (ICAPP 2021) (USB Flash Drive), 5 Pages, 2021/10

Impurity concentrations of hydrogen and hydride in the coolant were investigated in detail for the HTTR, a block type high-temperature gas reactor owned by Japan. As a result, it was found that CH$$_{4}$$ was 1/10 of H$$_{2}$$ concentration, which was under the conventional detection limit. If the ratio of H$$_{2}$$ to CH$$_{4}$$ in the coolant is the same as the ratio of HT to CH$$_{3}$$T, the CH$$_{3}$$T has a larger dose conversion factor, and this compositional ratio is an important finding for the optimal dose evaluation. Further investigation of the origin of CH$$_{4}$$ suggested that CH$$_{4}$$ was produced as a result of a thermal equilibrium reaction rather than being released as an impurity from the core.

Journal Articles

Proposal of evaluation method of graphite incombustibility

Hamamoto, Shimpei; Ohashi, Hirofumi; Iigaki, Kazuhiko; Shimazaki, Yosuke; Ono, Masato; Shimizu, Atsushi; Ishitsuka, Etsuo

Proceedings of 2021 International Congress on Advances in Nuclear Power Plants (ICAPP 2021) (USB Flash Drive), 6 Pages, 2021/10

Since the HTGR has a large amount of graphite material in the core, it is necessary to assume an accident in which the reactor pressure boundary is damaged and air flows into the core. It is important to state that at the time of this accident, graphite does not burn and the accident does not develop due to the heat of oxidation reaction. Therefore, in this study, in order to evaluate the combustibility of graphite materials, we propose a method to compare the calorific value and heat removal amount of the material. When calculating the calorific value, the structural material of HTTR, a high-temperature gas reactor in Japan, was used as a reference. The amount of air in contact with the structural material is a value determined from the chimney effect. The amount of heat release is the sum of convection and radiation. As a result of comparing the heat generation amount with the heat removal amount, it was shown that the heat release amount was always larger than the heat generation amount. This result shows that the graphite material does not depend on the state at the time of the air inflow accident, the temperature decreases and does not burn. It is important to clearly explain the non-flammability of graphite materials when deciding how to deal with severe accidents in HTGRs. This quantitative evaluation method based on a simple theory is considered useful.

Journal Articles

Formation of Type A glassy cesium-bearing microparticles from HEPA filter materials in Unit 3 during Fukushima Dai-ichi NPS accident; From viewpoint of similarity in silicate glass composition

Hidaka, Akihide

Proceedings of 2021 International Congress on Advances in Nuclear Power Plants (ICAPP 2021) (USB Flash Drive), 10 Pages, 2021/10

Author recently proposed that the Type A glassy Cesium-bearing microparticles that were released during the Fukushima accident may have been formed by melting and atomization of glass fibers of the High Efficiency Particulate Air (HEPA) filter in the Stand-by Gas Treatment System (SGTS) line in Unit 3 during the hydrogen explosion. In the present study, the components of the Type A and glass fibers of HEPA filter were examined using EPMA. The results showed that the components of the Type A were almost the same as that of the glass fibers except for Cs, Fe, Sn, which are considered to have been contained in the in-vessel-derived particles. When the glass fiber was irradiated with the electron beam of the Electron Probe Micro Analyzer (EPMA) under vacuum condition, spherical particles of a few micro m size were formed that looked very similar to the Type A. These strongly suggest that the HEPA filter is Si source of the Type A.

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